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High-speed free-run ptychography at the Australian Synchrotron

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posted on 2022-09-15, 06:57 authored by MWM Jones, Grant van RiessenGrant van Riessen, NW Phillips, CE Schrank, Gerard Hinsley, N Afshar, J Reinhardt, MD De Jonge, Cameron KewishCameron Kewish
Over the last decade ptychography has progressed rapidly from a specialist ultramicroscopy technique into a mature method accessible to non-expert users. However, to improve scientific value ptychography data must reconstruct reliably, with high image quality and at no cost to other correlative methods. Presented here is the implementation of high-speed ptychography used at the Australian Synchrotron on the XFM beamline, which includes a free-run data collection mode where dead time is eliminated and the scan time is optimized. It is shown that free-run data collection is viable for fast and high-quality ptychography by demonstrating extremely high data rate acquisition covering areas up to 352 000 μm2at up to 140 μm2s-1, with 13× spatial resolution enhancement compared with the beam size. With these improvements, ptychography at velocities up to 250 μm s-1is approaching speeds compatible with fast-scanning X-ray fluorescence microscopy. The combination of these methods provides morphological context for elemental and chemical information, enabling unique scientific outcomes.

Funding

The purchase of the EIGER2 detector was supported in part by an ARC Linkage Infrastructure, Equipment and Facilities (LIEF) grant (No. LE130100192). Christoph E. Schrank gratefully acknowledges funding by the Australian Research Council through a Discovery grant (No. DP170104550). NicholasW. Phillips acknowledges funding from the European Research Council (ERC) under the European Union Horizon 2020 research and innovation programme (grant agreement No. 714697) and under the Marie Sklodowska-Curie Actions (grant agreement No. 884104 PSI-FELLOW-III-3i).

History

Publication Date

2022-03-01

Journal

Journal of Synchrotron Radiation

Volume

29

Issue

Part 2

Pagination

8p. (p. 480-487)

Publisher

International Union of Crystallography

ISSN

0909-0495

Rights Statement

© The Authors 2022. This is deposited under the terms of the Creative Commons Attribution License: https://creativecommons.org/licenses/by/4.0/ You are free to share - copy and redistribute the material in any medium or format, and adapt - remix, transform, and build upon the material for any purpose, even commercially. The licensor cannot revoke these freedoms as long as you follow the license terms: i) attribution - you must give appropriate credit, provide a link to the license, and indicate if changes were made. You may do so in any reasonable manner, but not in any way that suggests the licensor endorses you or your use. ii) no additional restrictions - you may not apply legal terms or technological measures that legally restrict others from doing anything the license permits.